Electron Spin Resonance in the Double-Perovskite Oxide Antiferromagnet Ba2CoWO6

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • K. Yu Povarov - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR), Würzburg-Dresden Cluster of Excellence ct.qmat (Author)
  • J. Wosnitza - , Clusters of Excellence ct.qmat: Complexity and Topology in Quantum Matter, Chair of Physics of High Magnetic Fields, Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Author)
  • A. R.N. Hanna - , Technical University of Berlin, Helmholtz Centre Berlin for Materials and Energy (Author)
  • A. T.M.Nazmul Islam - , Helmholtz Centre Berlin for Materials and Energy (Author)
  • B. Lake - , Technical University of Berlin, Helmholtz Centre Berlin for Materials and Energy (Author)
  • S. A. Zvyagin - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR), Würzburg-Dresden Cluster of Excellence ct.qmat (Author)

Abstract

We report electron spin resonance studies of double perovskite Ba2CoWO6 single crystals. Above TN=14 K, we observe a paramagnetic resonance with geff≃3.66. Upon cooling, this mode transforms into a broad antiferromagnetic resonance (AFMR) with a zero-field energy gap of about 200 GHz. The AFMR becomes barely detectable at low magnetic fields, indicating unusually strong decay processes. We argue that symmetry-allowed anisotropic spin–spin interactions are a possible reason for the pronounced spin-wave damping. Linear spin-wave theory calculations support this scenario.

Details

Original languageEnglish
Pages (from-to)1549-1558
Number of pages10
JournalApplied Magnetic Resonance
Volume56
Issue number11
Early online date20 Oct 2025
Publication statusPublished - Nov 2025
Peer-reviewedYes

Keywords