Crystallization dynamics of amorphous yttrium iron garnet thin films

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Sebastian Sailler - , University of Konstanz (Author)
  • Gregor Skobjin - , University of Konstanz (Author)
  • Heike Schlörb - , Leibniz Institute for Solid State and Materials Research Dresden (Author)
  • Benny Boehm - , Chemnitz University of Technology (Author)
  • Olav Hellwig - , Chemnitz University of Technology (Author)
  • Andy Thomas - , Chair of Solid State Physics, Leibniz Institute for Solid State and Materials Research Dresden, TUD Dresden University of Technology (Author)
  • Sebastian T.B. Goennenwein - , University of Konstanz (Author)
  • Michaela Lammel - , University of Konstanz (Author)

Abstract

Yttrium iron garnet (YIG) is a prototypical material in spintronics due to its exceptional magnetic properties. To exploit these properties, high quality thin films need to be manufactured. Deposition techniques like sputter deposition or pulsed laser deposition at ambient temperature produce amorphous films, which need a postannealing step to induce crystallization. However, not much is known about the exact dynamics of the formation of crystalline YIG out of the amorphous phase. Here, we conduct extensive time and temperature series to study the crystallization behavior of YIG on various substrates and extract the crystallization velocities as well as the activation energies needed to promote crystallization. We find that the type of crystallization as well as the crystallization velocity depend on the lattice mismatch to the substrate. We compare the crystallization parameters found in literature with our results and find excellent agreement with our model. Our results allow us to determine the time needed for the formation of a fully crystalline film of arbitrary thickness for any temperature.

Details

Original languageEnglish
Article number043402
JournalPhysical review materials
Volume8
Issue number4
Publication statusPublished - Apr 2024
Peer-reviewedYes