Contrasting magnetic behavior in MnSc2X4 (X = S, Se) spinel compounds investigated by magnetoelastic studies

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Contributors

Abstract

The spinel compounds MnSc2X4 are highly frustrated and candidate materials for vortex-like 3q magnetic states, such as skyrmions, with propagation vectors in the [111] plane. Because of the strong magnetoelastic coupling, we could extract a refined magnetic (H,T) phase diagram for MnSc2S4 from ultrasound and dilatometry measurements. We found a variety of magnetic phases, including the skyrmion phase, which is stable down to lowest temperatures. In comparison, we investigated MnSc2Se4, having a larger distance between the magnetic Mn3+ ions using the same methods. Unlike in MnSc2S4, we found no skyrmion phase and overall a lack of sharp anomalies indicative of phase transitions, neither in dilatometry nor ultrasound nor in specific heat and ac-susceptibility data. Motivated by our findings, we performed model calculations, which reproduced the experimentally observed magnetostriction and specific-heat results reasonably well.

Details

Original languageEnglish
Article number214415
Number of pages9
JournalPhysical Review B
Volume112
Issue number21
Publication statusPublished - 8 Dec 2025
Peer-reviewedYes