Competing Exchange Interactions on the Verge of a Metal-Insulator Transition in the Two-Dimensional Spiral Magnet Sr3Fe2O7
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Contributors
Abstract
We report a neutron scattering study of the magnetic order and dynamics of the bilayer perovskite Sr3Fe2O7, which exhibits a temperature-driven metal-insulator transition at 340 K. We show that the Fe4+ moments adopt incommensurate spiral order below T-N = 115 K and provide a comprehensive description of the corresponding spin-wave excitations. The observed magnetic order and excitation spectra can be well understood in terms of an effective spin Hamiltonian with interactions ranging up to third-nearest-neighbor pairs. The results indicate that the helical magnetism in Sr3Fe2O7 results from competition between ferromagnetic double-exchange and antiferromagnetic superexchange interactions whose strengths become comparable near the metal-insulator transition. They thus confirm a decades-old theoretical prediction and provide a firm experimental basis for models of magnetic correlations in strongly correlated metals.
Details
Original language | English |
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Article number | 147206 |
Number of pages | 5 |
Journal | Physical review letters |
Volume | 113 |
Issue number | 14 |
Publication status | Published - 3 Oct 2014 |
Peer-reviewed | Yes |
Externally published | Yes |
External IDs
Scopus | 84908032090 |
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Keywords
Keywords
- CRYSTALS, SYSTEMS, ORDER