Breakdown of Hooke's law of elasticity at the mott critical endpoint in an organic conductor

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Elena Gati - , Goethe University Frankfurt a.M. (Author)
  • Markus Garst - , Chair of Theoretical Solid State Physics, University of Cologne, TUD Dresden University of Technology (Author)
  • Rudra S. Manna - , Goethe University Frankfurt a.M. (Author)
  • Ulrich Tutsch - , Goethe University Frankfurt a.M. (Author)
  • Bernd Wolf - , Goethe University Frankfurt a.M. (Author)
  • Lorenz Bartosch - , Goethe University Frankfurt a.M. (Author)
  • Harald Schubert - , Goethe University Frankfurt a.M. (Author)
  • Takahiko Sasaki - , Tohoku University (Author)
  • John A. Schlueter - , U.S. National Science Foundation, Argonne National Laboratory (Author)
  • Michael Lang - , Goethe University Frankfurt a.M. (Author)

Abstract

The Mott metal-insulator transition, a paradigm of strong electron-electron correlations, has been considered as a source of intriguing phenomena. Despite its importance for a wide range of materials, fundamental aspects of the transition, such as its universal properties, are still under debate. We report detailed measurements of relative length changes ΔL/L as a function of continuously controlled helium-gas pressure P for the organic conductor κ-(BEDT-TTF)2Cu[N(CN)2]Cl across the pressure-induced Mott transition. We observe strongly nonlinear variations of ΔL/L with pressure around the Mott critical endpoint, highlighting a breakdown of Hooke's law of elasticity. We assign these nonlinear strain-stress relations to an intimate, nonperturbative coupling of the critical electronic system to the lattice degrees of freedom. Our results are fully consistent with mean-field criticality, predicted for electrons in a compressible lattice with finite shear moduli. We argue that the Mott transition for all systems that are amenable to pressure tuning shows the universal properties of an isostructural solid-solid transition.

Details

Original languageEnglish
Article number1601646
JournalScience advances
Volume2
Issue number12
Publication statusPublished - Dec 2016
Peer-reviewedYes

Keywords

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