Adiabatic physics of an exchange-coupled spin-dimer system: Magnetocaloric effect, zero-point fluctuations, and possible two-dimensional universal behavior

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • J. Brambleby - , University of Warwick (Author)
  • P. A. Goddard - , University of Warwick (Author)
  • J. Singleton - , National High Magnetic Field Laboratory Los Almos (Author)
  • M. Jaime - , National High Magnetic Field Laboratory Los Almos (Author)
  • T. Lancaster - , Durham University (Author)
  • L. Huang - , Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • J. Wosnitza - , Chair of Physics of High Magnetic Fields, Helmholtz-Zentrum Dresden-Rossendorf (Author)
  • C. V. Topping - , University of Oxford (Author)
  • K. E. Carreiro - , Eastern Washington University (Author)
  • H. E. Tran - , Eastern Washington University (Author)
  • Z. E. Manson - , Eastern Washington University (Author)
  • J. L. Manson - , Eastern Washington University (Author)

Abstract

We present the magnetic and thermal properties of the bosonic-superfluid phase in a spin-dimer network using both quasistatic and rapidly changing pulsed magnetic fields. The entropy derived from a heat-capacity study reveals that the pulsed-field measurements are strongly adiabatic in nature and are responsible for the onset of a significant magnetocaloric effect (MCE). In contrast to previous predictions we show that the MCE is not just confined to the critical regions, but occurs for all fields greater than zero at sufficiently low temperatures. We explain the MCE using a model of the thermal occupation of exchange-coupled dimer spin states and highlight that failure to take this effect into account inevitably leads to incorrect interpretations of experimental results. In addition, the heat capacity in our material is suggestive of an extraordinary contribution from zero-point fluctuations and appears to indicate universal behavior with different critical exponents at the two field-induced critical points. The data at the upper critical point, combined with the layered structure of the system, are consistent with a two-dimensional nature of spin excitations in the system.

Details

Original languageEnglish
Article number024404
JournalPhysical Review B
Volume95
Issue number2
Publication statusPublished - 5 Jan 2017
Peer-reviewedYes