The Role of Electronic and Phononic Excitation in the Optical Response of Monolayer WS2 after Ultrafast Excitation

Publikation: Beitrag in FachzeitschriftForschungsartikelBeigetragenBegutachtung

Beitragende

  • Claudia Ruppert - , Columbia University, Technische Universität (TU) Dortmund (Autor:in)
  • Alexey Chernikov - , Columbia University, Universität Regensburg (Autor:in)
  • Heather M. Hill - , Columbia University, Stanford University, Stanford Linear Accelerator Center (SLAC) (Autor:in)
  • Albert F. Rigosi - , Columbia University, Stanford University, Stanford Linear Accelerator Center (SLAC) (Autor:in)
  • Tony F. Heinz - , Columbia University, Stanford University, Stanford Linear Accelerator Center (SLAC) (Autor:in)

Abstract

Transient changes of the optical response of WS2 monolayers are studied by femtosecond broadband pump-probe spectroscopy. Time-dependent absorption spectra are analyzed by tracking the line width broadening, bleaching, and energy shift of the main exciton resonance as a function of time delay after the excitation. Two main sources for the pump-induced changes of the optical response are identified. Specifically, we find an interplay between modifications induced by many-body interactions from photoexcited carriers and by the subsequent transfer of the excitation to the phonon system followed by cooling of the material through the heat transfer to the substrate.

Details

OriginalspracheEnglisch
Seiten (von - bis)644-651
Seitenumfang8
FachzeitschriftNano letters
Jahrgang17
Ausgabenummer2
PublikationsstatusVeröffentlicht - 8 Feb. 2017
Peer-Review-StatusJa
Extern publiziertJa

Externe IDs

PubMed 28059520

Schlagworte

Schlagwörter

  • Atomically thin 2D materials, carrier and phonon dynamics, ultrafast spectroscopy