Valley-magnetophonon resonance for interlayer excitons

Publikation: Beitrag in FachzeitschriftForschungsartikelBeigetragenBegutachtung

Beitragende

  • Dmitry S. Smirnov - , RAS - Ioffe Physico Technical Institute, St. Petersburg State University (Autor:in)
  • Johannes Holler - , Universität Regensburg (Autor:in)
  • Michael Kempf - , Universität Rostock (Autor:in)
  • Jonas Zipfel - , Universität Regensburg, Lawrence Berkeley National Laboratory (Autor:in)
  • Philipp Nagler - , Universität Regensburg (Autor:in)
  • Mariana V. Ballottin - , Radboud University Nijmegen (Autor:in)
  • Anatolie A. Mitioglu - , Radboud University Nijmegen (Autor:in)
  • Alexey Chernikov - , Professur für Ultraschnelle Mikroskopie und Photonik (ct.qmat), Exzellenzcluster ct.qmat: Komplexität und Topologie in Quantenmaterialien, Universität Regensburg (Autor:in)
  • Peter C.M. Christianen - , Radboud University Nijmegen (Autor:in)
  • Christian Schüller - , Universität Regensburg (Autor:in)
  • Tobias Korn - , Universität Rostock (Autor:in)

Abstract

Heterobilayers consisting of MoSe2 and WSe2 monolayers can host optically bright interlayer excitons with intriguing properties such as ultralong lifetimes and pronounced circular polarization of their photoluminescence due to valley polarization, which can be induced by circularly polarized excitation or applied magnetic fields. Here, we report on the observation of an intrinsic valley-magnetophonon resonance for localized interlayer excitons promoted by invervalley hole scattering. It leads to a resonant increase of the photoluminescence polarization degree at the same field of 24.2 Tesla for H-type and R-type stacking configurations despite their vastly different excitonic energy splittings. As a microscopic mechanism of the hole intervalley scattering we identify the scattering with chiral TA phonons of MoSe2 between excitonic states mixed by the long-range electron hole exchange interaction.

Details

OriginalspracheEnglisch
Aufsatznummer045016
Fachzeitschrift2D materials
Jahrgang9
Ausgabenummer4
PublikationsstatusVeröffentlicht - Okt. 2022
Peer-Review-StatusJa

Schlagworte

Schlagwörter

  • excitons, heterobilayer, intervalley scattering, magnetophonon resonance, photoluminescence, transition metal dichalcogenide

Bibliotheksschlagworte