Self-Driven Broadband Photodetectors Based on MoSe2/FePS3 van der Waals n-p Type-II Heterostructures

Publikation: Beitrag in FachzeitschriftForschungsartikelBeigetragenBegutachtung

Beitragende

  • Juanmei Duan - , Professur für Spektroskopie in der Halbleiterphysik (gB/HZDR), Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Autor:in)
  • Phanish Chava - , Professur für Nanoelektronik, Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Autor:in)
  • Mahdi Ghorbani-Asl - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Autor:in)
  • Yang Fan Lu - , Zhejiang University (Autor:in)
  • Denise Erb - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Autor:in)
  • Liang Hu - , Hangzhou Dianzi University, Zhejiang University (Autor:in)
  • Ahmad Echresh - , Professur für Spektroskopie in der Halbleiterphysik (gB/HZDR), Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Autor:in)
  • Lars Rebohle - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Autor:in)
  • Artur Erbe - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Autor:in)
  • Arkady V. Krasheninnikov - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR), Aalto University (Autor:in)
  • Manfred Helm - , Professur für Spektroskopie in der Halbleiterphysik (gB/HZDR), Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Autor:in)
  • Yu Jia Zeng - , Shenzhen University (Autor:in)
  • Shengqiang Zhou - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Autor:in)
  • Slawomir Prucnal - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Autor:in)

Abstract

Two-dimensional (2D) van der Waals materials with broadband optical absorption are promising candidates for next-generation UV-vis-NIR photodetectors. FePS3, one of the emerging antiferromagnetic van der Waals materials with a wide bandgap and p-type conductivity, has been reported as an excellent candidate for UV optoelectronics. However, a high sensitivity photodetector with a self-driven mode based on FePS3 has not yet been realized. Here, we report a high-performance and self-powered photodetector based on a multilayer MoSe2/FePS3 type-II n-p heterojunction with a working range from 350 to 900 nm. The presented photodetector operates at zero bias and at room temperature under ambient conditions. It exhibits a maximum responsivity (Rmax) of 52 mA W-1 and an external quantum efficiency (EQEmax) of 12% at 522 nm, which are better than the characteristics of its individual constituents and many other photodetectors made of 2D heterostructures. The high performance of MoSe2/FePS3 is attributed to the built-in electric field in the MoSe2/FePS3 n-p junction. Our approach provides a promising platform for broadband self-driven photodetector applications.

Details

OriginalspracheEnglisch
Seiten (von - bis)11927-11936
Seitenumfang10
FachzeitschriftACS Applied Materials and Interfaces
Jahrgang14
Ausgabenummer9
PublikationsstatusVeröffentlicht - 9 März 2022
Peer-Review-StatusJa

Externe IDs

PubMed 35191687

Schlagworte

ASJC Scopus Sachgebiete

Schlagwörter

  • broadband photodetector, iron phosphorus trisulfide, molybdenum diselenide, type-II band alignment, van der Waals heterojunction

Bibliotheksschlagworte