Self-Driven Broadband Photodetectors Based on MoSe2/FePS3 van der Waals n-p Type-II Heterostructures
Publikation: Beitrag in Fachzeitschrift › Forschungsartikel › Beigetragen › Begutachtung
Beitragende
Abstract
Two-dimensional (2D) van der Waals materials with broadband optical absorption are promising candidates for next-generation UV-vis-NIR photodetectors. FePS3, one of the emerging antiferromagnetic van der Waals materials with a wide bandgap and p-type conductivity, has been reported as an excellent candidate for UV optoelectronics. However, a high sensitivity photodetector with a self-driven mode based on FePS3 has not yet been realized. Here, we report a high-performance and self-powered photodetector based on a multilayer MoSe2/FePS3 type-II n-p heterojunction with a working range from 350 to 900 nm. The presented photodetector operates at zero bias and at room temperature under ambient conditions. It exhibits a maximum responsivity (Rmax) of 52 mA W-1 and an external quantum efficiency (EQEmax) of 12% at 522 nm, which are better than the characteristics of its individual constituents and many other photodetectors made of 2D heterostructures. The high performance of MoSe2/FePS3 is attributed to the built-in electric field in the MoSe2/FePS3 n-p junction. Our approach provides a promising platform for broadband self-driven photodetector applications.
Details
| Originalsprache | Englisch |
|---|---|
| Seiten (von - bis) | 11927-11936 |
| Seitenumfang | 10 |
| Fachzeitschrift | ACS Applied Materials and Interfaces |
| Jahrgang | 14 |
| Ausgabenummer | 9 |
| Publikationsstatus | Veröffentlicht - 9 März 2022 |
| Peer-Review-Status | Ja |
Externe IDs
| PubMed | 35191687 |
|---|
Schlagworte
ASJC Scopus Sachgebiete
Schlagwörter
- broadband photodetector, iron phosphorus trisulfide, molybdenum diselenide, type-II band alignment, van der Waals heterojunction