Observation of excitonic rydberg states in monolayer MoS2 and WS2 by photoluminescence excitation spectroscopy

Publikation: Beitrag in FachzeitschriftForschungsartikelBeigetragenBegutachtung

Beitragende

  • Heather M. Hill - , Columbia University (Autor:in)
  • Albert F. Rigosi - , Columbia University (Autor:in)
  • Cyrielle Roquelet - , Columbia University (Autor:in)
  • Alexey Chernikov - , Columbia University (Autor:in)
  • Timothy C. Berkelbach - , Columbia University (Autor:in)
  • David R. Reichman - , Columbia University (Autor:in)
  • Mark S. Hybertsen - , Brookhaven National Laboratory (Autor:in)
  • Louis E. Brus - , Columbia University (Autor:in)
  • Tony F. Heinz - , Columbia University (Autor:in)

Abstract

We have identified excited exciton states in monolayers of MoS2 and WS2 supported on fused silica by means of photoluminescence excitation spectroscopy. In monolayer WS2, the positions of the excited A exciton states imply an exciton binding energy of 0.32 eV. In monolayer MoS2, excited exciton transitions are observed at energies of 2.24 and 2.34 eV. Assigning these states to the B exciton Rydberg series yields an exciton binding energy of 0.44 eV.

Details

OriginalspracheEnglisch
Seiten (von - bis)2992-2997
Seitenumfang6
FachzeitschriftNano letters
Jahrgang15
Ausgabenummer5
PublikationsstatusVeröffentlicht - 13 Mai 2015
Peer-Review-StatusJa
Extern publiziertJa

Externe IDs

PubMed 25816155

Schlagworte

Schlagwörter

  • 2D materials, binding energy, excitons, molybdenum disulfide, Transition metal dichalcogenides, tungsten disulfide