Exciton Propagation and Halo Formation in Two-Dimensional Materials

Publikation: Beitrag in FachzeitschriftForschungsartikelBeigetragenBegutachtung

Beitragende

  • Raül Perea-Causín - , Chalmers University of Technology (Autor:in)
  • Samuel Brem - , Chalmers University of Technology (Autor:in)
  • Roberto Rosati - , Chalmers University of Technology (Autor:in)
  • Roland Jago - , Chalmers University of Technology (Autor:in)
  • Marvin Kulig - , Universität Regensburg (Autor:in)
  • Jonas D. Ziegler - , Universität Regensburg (Autor:in)
  • Jonas Zipfel - , Universität Regensburg (Autor:in)
  • Alexey Chernikov - , Universität Regensburg (Autor:in)
  • Ermin Malic - , Chalmers University of Technology (Autor:in)

Abstract

The interplay of optics, dynamics, and transport is crucial for the design of novel optoelectronic devices, such as photodetectors and solar cells. In this context, transition-metal dichalcogenides (TMDs) have received much attention. Here, strongly bound excitons dominate optical excitation, carrier dynamics, and diffusion processes. While the first two have been intensively studied, there is a lack of fundamental understanding of nonequilibrium phenomena associated with exciton transport that is of central importance (e.g., for high-efficiency light harvesting). In this work, we provide microscopic insights into the interplay of exciton propagation and many-particle interactions in TMDs. On the basis of a fully quantum mechanical approach and in excellent agreement with photoluminescence measurements, we show that Auger recombination and emission of hot phonons act as a heating mechanism giving rise to strong spatial gradients in excitonic temperature. The resulting thermal drift leads to an unconventional exciton diffusion characterized by spatial exciton halos.

Details

OriginalspracheEnglisch
Seiten (von - bis)7317-7323
Seitenumfang7
FachzeitschriftNano letters
Jahrgang19
Ausgabenummer10
PublikationsstatusVeröffentlicht - 9 Okt. 2019
Peer-Review-StatusJa
Extern publiziertJa

Externe IDs

PubMed 31532993

Schlagworte

Schlagwörter

  • Auger scattering, exciton diffusion, halos, hot phonons