Electronic superlattice revealed by resonant scattering from random impurities in Sr3Ru2O7
Publikation: Beitrag in Fachzeitschrift › Forschungsartikel › Beigetragen › Begutachtung
Beitragende
Abstract
Resonant elastic x-ray scattering (REXS) is an exquisite element-sensitive tool for the study of subtle charge, orbital, and spin superlattice orders driven by the valence electrons, which therefore escape detection in conventional x-ray diffraction (XRD). Although the power of REXS has been demonstrated by numerous studies of complex oxides performed in the soft x-ray regime, the cross section and photon wavelength of the material-specific elemental absorption edges ultimately set the limit to the smallest superlattice amplitude and periodicity one can probe. Here we show - with simulations and REXS on Mn-substituted Sr3Ru2O7 - that these limitations can be overcome by performing resonant scattering experiments at the absorption edge of a suitably-chosen, dilute impurity. This establishes that - in analogy with impurity-based methods used in electron-spin-resonance, nuclear-magnetic resonance, and Mössbauer spectroscopy - randomly distributed impurities can serve as a non-invasive, but now momentum-dependent probe, greatly extending the applicability of resonant x-ray scattering techniques.
Details
Originalsprache | Englisch |
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Aufsatznummer | 2299 |
Fachzeitschrift | Scientific reports |
Jahrgang | 3 |
Publikationsstatus | Veröffentlicht - 2013 |
Peer-Review-Status | Ja |
Externe IDs
PubMed | 23903555 |
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ORCID | /0000-0002-2438-0672/work/159172179 |