Electronic superlattice revealed by resonant scattering from random impurities in Sr3Ru2O7

Publikation: Beitrag in FachzeitschriftForschungsartikelBeigetragenBegutachtung

Beitragende

  • M. A. Hossain - , University of British Columbia, United States Department of Energy (Autor:in)
  • I. Zegkinoglou - , Max-Planck-Institut für Festkörperforschung (Autor:in)
  • Y. D. Chuang - , United States Department of Energy (Autor:in)
  • J. Geck - , Professur für Physik der Quantenmaterialien, University of British Columbia (Autor:in)
  • B. Bohnenbuck - , Max-Planck-Institut für Festkörperforschung (Autor:in)
  • A. G.Cruz Gonzalez - , United States Department of Energy (Autor:in)
  • H. H. Wu - , Universität zu Köln (Autor:in)
  • C. Schüßler-Langeheine - , Universität zu Köln (Autor:in)
  • D. G. Hawthorn - , University of British Columbia (Autor:in)
  • J. D. Denlinger - , United States Department of Energy (Autor:in)
  • R. Mathieu - , The University of Tokyo (Autor:in)
  • Y. Tokura - , The University of Tokyo (Autor:in)
  • S. Satow - , The University of Tokyo (Autor:in)
  • H. Takagi - , The University of Tokyo (Autor:in)
  • Y. Yoshida - , National Institute of Advanced Industrial Science and Technology (Autor:in)
  • Z. Hussain - , United States Department of Energy (Autor:in)
  • B. Keimer - , Max-Planck-Institut für Festkörperforschung (Autor:in)
  • G. A. Sawatzky - , University of British Columbia (Autor:in)
  • A. Damascelli - , University of British Columbia (Autor:in)

Abstract

Resonant elastic x-ray scattering (REXS) is an exquisite element-sensitive tool for the study of subtle charge, orbital, and spin superlattice orders driven by the valence electrons, which therefore escape detection in conventional x-ray diffraction (XRD). Although the power of REXS has been demonstrated by numerous studies of complex oxides performed in the soft x-ray regime, the cross section and photon wavelength of the material-specific elemental absorption edges ultimately set the limit to the smallest superlattice amplitude and periodicity one can probe. Here we show - with simulations and REXS on Mn-substituted Sr3Ru2O7 - that these limitations can be overcome by performing resonant scattering experiments at the absorption edge of a suitably-chosen, dilute impurity. This establishes that - in analogy with impurity-based methods used in electron-spin-resonance, nuclear-magnetic resonance, and Mössbauer spectroscopy - randomly distributed impurities can serve as a non-invasive, but now momentum-dependent probe, greatly extending the applicability of resonant x-ray scattering techniques.

Details

OriginalspracheEnglisch
Aufsatznummer2299
FachzeitschriftScientific reports
Jahrgang3
PublikationsstatusVeröffentlicht - 2013
Peer-Review-StatusJa

Externe IDs

PubMed 23903555
ORCID /0000-0002-2438-0672/work/159172179

Schlagworte

ASJC Scopus Sachgebiete