Electrically powered repeatable air explosions using microtubular graphene assemblies

Publikation: Beitrag in FachzeitschriftForschungsartikelBeigetragenBegutachtung

Beitragende

  • Fabian Schütt - , Christian-Albrechts-Universität zu Kiel (CAU) (Autor:in)
  • Florian Rasch - , Christian-Albrechts-Universität zu Kiel (CAU) (Autor:in)
  • Nipon Deka - , Christian-Albrechts-Universität zu Kiel (CAU) (Autor:in)
  • Armin Reimers - , Christian-Albrechts-Universität zu Kiel (CAU) (Autor:in)
  • Lena M. Saure - , Christian-Albrechts-Universität zu Kiel (CAU) (Autor:in)
  • Sören Kaps - , Christian-Albrechts-Universität zu Kiel (CAU) (Autor:in)
  • Jannik Rank - , Christian-Albrechts-Universität zu Kiel (CAU) (Autor:in)
  • Jürgen Carstensen - , Christian-Albrechts-Universität zu Kiel (CAU) (Autor:in)
  • Yogendra Kumar Mishra - , University of Southern Denmark (Autor:in)
  • Diego Misseroni - , Università degli Studi di Trento (Autor:in)
  • Adrian Romani Vázquez - , Professur für Molekulare Funktionsmaterialien (cfaed) (Autor:in)
  • Martin R. Lohe - , Professur für Molekulare Funktionsmaterialien (cfaed), Sixonia Tech GmbH (Autor:in)
  • Ali Shaygan Nia - , Professur für Molekulare Funktionsmaterialien (cfaed) (Autor:in)
  • Nicola M. Pugno - , Università degli Studi di Trento, Queen Mary University of London (Autor:in)
  • Xinliang Feng - , Professur für Molekulare Funktionsmaterialien (cfaed) (Autor:in)
  • Rainer Adelung - , Christian-Albrechts-Universität zu Kiel (CAU) (Autor:in)

Abstract

Controllable rapid expansion and activation of gases is important for a variety of applications, including combustion engines, thrusters, actuators, catalysis, and sensors. Typically, the activation of macroscopic gas volumes is based on ultra-fast chemical reactions, which require fuel and are irreversible. An “electrically powered explosion”, i.e., the rapid increase in temperature of a macroscopic relevant gas volume induced by an electrical power pulse, is a feasible repeatable and clean alternative, providing adaptable non-chemical power on demand. Till now, the fundamental problem was to find an efficient transducer material that converts electrical energy into an immediate temperature increase of a sufficient gas volume. To overcome these limitations, we developed electrically powered repeatable air explosions (EPRAE) based on free-standing graphene layers of nanoscale thickness in the form of microtubes that are interconnected to a macroscopic framework. These low-density and highly permeable graphene foams are characterized by heat capacities comparable to air. The EPRAE process facilitates cyclic heating of cm3-sized air volumes to several 100 °C for more than 100,000 cycles, heating rates beyond 300,000 K s−1 and repetition rates of several Hz. It enables pneumatic actuators with the highest observed output power densities (>40 kW kg−1) and strains ∼100%, as well as tunable microfluidic pumps, gas flowmeters, thermophones, and micro-thrusters.

Details

OriginalspracheEnglisch
Seiten (von - bis)7-17
Seitenumfang11
FachzeitschriftMaterials today
Jahrgang48
PublikationsstatusVeröffentlicht - Sept. 2021
Peer-Review-StatusJa