Clocking the melting transition of charge and lattice order in 1T-TaS 2 with ultrafast extreme-ultraviolet angle-resolved photoemission spectroscopy

Publikation: Beitrag in FachzeitschriftForschungsartikelBeigetragenBegutachtung

Beitragende

  • J. C. Petersen - , University of Oxford, Universität Hamburg (Autor:in)
  • S. Kaiser - , Max Planck Institute for the Structure and Dynamics of Matter, Universität Hamburg (Autor:in)
  • N. Dean - , Universität Hamburg (Autor:in)
  • A. Simoncig - , Universität Hamburg (Autor:in)
  • H. Y. Liu - , Universität Hamburg (Autor:in)
  • A. L. Cavalieri - , Universität Hamburg (Autor:in)
  • C. Cacho - , Rutherford Appleton Laboratory (Autor:in)
  • I. C.E. Turcu - , Rutherford Appleton Laboratory (Autor:in)
  • E. Springate - , Rutherford Appleton Laboratory (Autor:in)
  • F. Frassetto - , National Research Council of Italy (CNR) (Autor:in)
  • L. Poletto - , National Research Council of Italy (CNR) (Autor:in)
  • S. S. Dhesi - , Diamond Light Source (Autor:in)
  • H. Berger - , École Polytechnique Fédérale de Lausanne (Autor:in)
  • A. Cavalleri - , University of Oxford, Universität Hamburg (Autor:in)

Abstract

We use time- and angle-resolved photoemission spectroscopy with sub-30-fs extreme-ultraviolet pulses to map the time- and momentum-dependent electronic structure of photoexcited 1T-TaS2. This compound is a two-dimensional Mott insulator with charge-density wave ordering. Charge order, evidenced by splitting between occupied subbands at the Brillouin zone boundary, melts well before the lattice responds. This challenges the view of a charge-density wave caused by electron-phonon coupling and Fermi-surface nesting alone, and suggests that electronic correlations play a key role in driving charge order.

Details

OriginalspracheEnglisch
Aufsatznummer177402
FachzeitschriftPhysical review letters
Jahrgang107
Ausgabenummer17
PublikationsstatusVeröffentlicht - 18 Okt. 2011
Peer-Review-StatusJa
Extern publiziertJa

Externe IDs

ORCID /0000-0001-9862-2788/work/142255388

Schlagworte

ASJC Scopus Sachgebiete