Clocking the melting transition of charge and lattice order in 1T-TaS 2 with ultrafast extreme-ultraviolet angle-resolved photoemission spectroscopy
Publikation: Beitrag in Fachzeitschrift › Forschungsartikel › Beigetragen › Begutachtung
Beitragende
Abstract
We use time- and angle-resolved photoemission spectroscopy with sub-30-fs extreme-ultraviolet pulses to map the time- and momentum-dependent electronic structure of photoexcited 1T-TaS2. This compound is a two-dimensional Mott insulator with charge-density wave ordering. Charge order, evidenced by splitting between occupied subbands at the Brillouin zone boundary, melts well before the lattice responds. This challenges the view of a charge-density wave caused by electron-phonon coupling and Fermi-surface nesting alone, and suggests that electronic correlations play a key role in driving charge order.
Details
Originalsprache | Englisch |
---|---|
Aufsatznummer | 177402 |
Fachzeitschrift | Physical review letters |
Jahrgang | 107 |
Ausgabenummer | 17 |
Publikationsstatus | Veröffentlicht - 18 Okt. 2011 |
Peer-Review-Status | Ja |
Extern publiziert | Ja |
Externe IDs
ORCID | /0000-0001-9862-2788/work/142255388 |
---|