Bias-Free Access to Orbital Angular Momentum in Two-Dimensional Quantum Materials

Publikation: Beitrag in FachzeitschriftForschungsartikelBeigetragenBegutachtung

Beitragende

  • Jonas Erhardt - , Julius-Maximilians-Universität Würzburg (Autor:in)
  • Cedric Schmitt - , Julius-Maximilians-Universität Würzburg (Autor:in)
  • Philipp Eck - , Julius-Maximilians-Universität Würzburg (Autor:in)
  • Matthias Schmitt - , Julius-Maximilians-Universität Würzburg, Diamond Light Source (Autor:in)
  • Philipp Keßler - , Julius-Maximilians-Universität Würzburg (Autor:in)
  • Kyungchan Lee - , Julius-Maximilians-Universität Würzburg (Autor:in)
  • Timur Kim - , Diamond Light Source (Autor:in)
  • Cephise Cacho - , Diamond Light Source (Autor:in)
  • Iulia Cojocariu - , Sincrotrone Trieste, Forschungszentrum Jülich, Università degli Studi di Trieste (Autor:in)
  • Daniel Baranowski - , Forschungszentrum Jülich (Autor:in)
  • Vitaliy Feyer - , Forschungszentrum Jülich, Universität Duisburg-Essen (Autor:in)
  • Louis Veyrat - , Julius-Maximilians-Universität Würzburg, Leibniz-Institut für Festkörper- und Werkstoffforschung Dresden, Centre national de la recherche scientifique (CNRS), Würzburg-Dresden Cluster of Excellence ct.qmat (Autor:in)
  • Giorgio Sangiovanni - , Julius-Maximilians-Universität Würzburg (Autor:in)
  • Ralph Claessen - , Julius-Maximilians-Universität Würzburg (Autor:in)
  • Simon Moser - , Julius-Maximilians-Universität Würzburg (Autor:in)

Abstract

The demonstration of a topological band inversion constitutes the most elementary proof of a quantum spin Hall insulator (QSHI). On a fundamental level, such an inverted band gap is intrinsically related to the bulk Berry curvature, a gauge-invariant fingerprint of the wave function's quantum geometric properties in Hilbert space. Intimately tied to orbital angular momentum (OAM), the Berry curvature can be, in principle, extracted from circular dichroism in angle-resolved photoemission spectroscopy (CD-ARPES), were it not for interfering final state photoelectron emission channels that obscure the initial state OAM signature. Here, we outline a full-experimental strategy to avoid such interference artifacts and isolate the clean OAM from the CD-ARPES response. Bench-marking this strategy for the recently discovered atomic monolayer system indenene, we demonstrate its distinct QSHI character and establish CD-ARPES as a scalable bulk probe to experimentally classify the topology of two-dimensional quantum materials with time reversal symmetry.

Details

OriginalspracheEnglisch
Aufsatznummer196401
FachzeitschriftPhysical review letters
Jahrgang132
Ausgabenummer19
PublikationsstatusVeröffentlicht - 10 Mai 2024
Peer-Review-StatusJa

Schlagworte

ASJC Scopus Sachgebiete