Giant quantum oscillations in thermal transport in low-density metals via electron absorption of phonons

Research output: Contribution to journalResearch articleContributedpeer-review

Contributors

  • Baptiste Bermond - , Physics Laboratory of the ENS Lyon (Author)
  • Rafał Wawrzyńczak - , Max Planck Institute for Chemical Physics of Solids (Author)
  • Sergei Zherlitsyn - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Author)
  • Tommy Kotte - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Author)
  • Toni Helm - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Author)
  • Denis Gorbunov - , Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Author)
  • Genda Gu - , Brookhaven National Laboratory, Stony Brook University (Author)
  • Qiang Li - , Stony Brook University (Author)
  • Filip Janasz - , University of Luxembourg (Author)
  • Tobias Meng - , Clusters of Excellence ct.qmat: Complexity and Topology in Quantum Matter, Chair of Theoretical Solid State Physics (Author)
  • Fabian Menges - , Max Planck Institute for Chemical Physics of Solids (Author)
  • Claudia Felser - , Max Planck Institute for Chemical Physics of Solids (Author)
  • Joachim Wosnitza - , Clusters of Excellence ct.qmat: Complexity and Topology in Quantum Matter, Chair of Physics of High Magnetic Fields, Helmholtz-Zentrum Dresden-Rossendorf (HZDR) (Author)
  • Adolfo Grushin - , Université Grenoble Alpes (Author)
  • David Carpentier - , Physics Laboratory of the ENS Lyon (Author)
  • Johannes Gooth - , Max Planck Institute for Chemical Physics of Solids, University of Bonn (Author)
  • Stanisław Gałeski - , Max Planck Institute for Chemical Physics of Solids, Helmholtz-Zentrum Dresden-Rossendorf (HZDR), University of Bonn (Author)

Abstract

Oscillations of conductance observed in strong magnetic fields are a striking manifestation of the quantum dynamics of charge carriers in solids. The large charge carrier density in typical metals sets the scale of oscillations in both electrical and thermal conductivity, which characterize the Fermi surface. In semimetals, thermal transport at low-charge carrier density is expected to be phonon dominated, yet several experiments observe giant quantum oscillations in thermal transport. This raises the question of whether there is an overarching mechanism leading to sizable oscillations that survives in phonon-dominated semimetals. In this work, we show that such a mechanism exists. It relies on the peculiar phase-space allowed for phonon scattering by electrons when only a few Landau levels are filled. Our measurements on the Dirac semimetal ZrTe5 support this counterintuitive mechanism through observation of pronounced thermal quantum oscillations, since they occur in similar magnitude and phase in directions parallel and transverse to the magnetic field. Our phase-space argument applies to all low-density semimetals, topological or not, including graphene and bismuth. Our work illustrates that phonon absorption can be leveraged to reveal degrees of freedom through their imprint on longitudinal thermal transport.

Details

Original languageEnglish
Article numbere2408546122
JournalProceedings of the National Academy of Sciences of the United States of America
Volume122
Issue number10
Publication statusPublished - 11 Mar 2025
Peer-reviewedYes

External IDs

PubMed 40042911

Keywords

ASJC Scopus subject areas

Keywords

  • Dirac semimetal, Landau levels, quantum limit, thermal transport, Wiedemann–Franz law